Through simulation and experiments, the influences of container sizes on the machining effectiveness of cylindrical rollers in vertical vibration superfinishing rolling processes were investigated. The relation among the dimensional parameters and the movement characteristics of rollers and the mechanical behavior of surface particles was analyzed with the angle α and size d of “reverse L-container” as variables. With the increase of α, the height of the roller active region decreased gradually, and the deviation degree between the axis and the horizontal plane decreases first and then increased. The normal contact force of the outer diameter surface increased first and then decreased, while the tangential relative velocity decreased gradually. The normal contact force decreased first and then increased, while the tangential relative velocity increased first and then decreased. With the increase of d, the height of the rollers active region gradually increased, the deviation degree between the axis and the horizontal plane first decreased and then increased, the normal contact force of the outer diameter surface first increased and then decreased, the normal contact force of the end face first decreased and then increased, and the tangential relative velocity of the outer diameter surface and the end face increased gradually. The experimental results agree with the simulation results. The better container size:α=10°, d=50 mm, after processing, the outer diameter surface roughness value is reduced from 0.105 μm to 0.036 μm, the end surface roughness value is reduced from 0.150 μm to 0.057 μm, the surface profile is flat relatively, and the scratches are removed basically.